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One of my favourite moments from the game, is when you do the duel at the beginning, the music is great, but my all time favourite scene, would have to be when Bahamut is first summoned by the Queen and it completely destroys here fleet and actually manages to hurt Kuja ^-^
I absolutely agree. That mash-button scene thing with Blank was awesome! And yeah, it helped that the music was catchy too.
I also enjoyed very much the battle for Alexandria were you're running through what I'm guessing is the main street, hacking your way through with Beatrix and Steiner. And when you complete that, you're awarded with an awesome cut scene.